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Title: FORCED PERIODIC OPERATION OF TUBULAR REACTORS
Creator: Ozgulsen, F., Cinar, A.
Date: 1994-10
Publisher: PERGAMON-ELSEVIER SCIENCE LTD
Description: Forced periodic operation of tubular reactors can increase conversion and yield if proper operating conditions and forcing policies are...
Show moreForced periodic operation of tubular reactors can increase conversion and yield if proper operating conditions and forcing policies are selected. A numerical approach is proposed for computing the effects of periodic input forcing by a shooting algorithm. Such computational tools permit the assessment of the benefits of forced periodic operation of a specific reactor system and the identification of the ranges of operating conditions where forced periodic operation is beneficial. This information provides valuable insight for planning detailed experimental studies. Determining the influential input variables and bracketing the ranges of the operating conditions for improving reactor performance will reduce significantly the experiments needed for selecting the most favorable reactor operation policies. The application of the numerical algorithm is illustrated by assessing the benefits of forced periodic operation to a CO oxidation reactor model. The results reveal substantial improvement in performance with slow cycling in feed concentration.
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Title: A NUMERICAL-METHOD FOR DETERMINING OPTIMAL PARAMETER VALUES IN FORCED PERIODIC OPERATION
Creator: Ozgulsen, F., Adomaitis, R. A., Cinar, A.
Date: 1992-02
Publisher: PERGAMON-ELSEVIER SCIENCE LTD
Description: A numerical approach for determining values of forcing parameters which maximize performance of a periodically forced system is described....
Show moreA numerical approach for determining values of forcing parameters which maximize performance of a periodically forced system is described. Periodic solutions of the system equations plus a differential form of the time-average performance measure are computed with a shooting algorithm. A nonlinear programming package is used to solve the optimization problem. The algorithm is applied to ethylene oxidation process, using the model of a continuous stirred-tank reactor (CSTR).
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Title: NONLINEAR PREDICTIVE CONTROL OF PERIODICALLY FORCED CHEMICAL REACTORS
Creator: Ozgulsen, F., Kendra, S. J., Cinar, A.
Date: 1993-04
Publisher: AMER INST CHEMICAL ENGINEERS
Description: A nonlinear model-predictive control strategy is developed to maintain the superior-to-steady-state performance of a periodically forced...
Show moreA nonlinear model-predictive control strategy is developed to maintain the superior-to-steady-state performance of a periodically forced chemical reactor. The performance of the predictive con troller is investigated in the presence of measurement disturbances and parametric uncertainty. It is also shown that statistically inferred input-output models can be a substitute whenever detailed fundamental models are not available. A nonlinear autoregressive polynomial model based on observed plant data is built and incorporated into the control scheme. The catalytic oxidation of ethylene in a periodically-forced, continuous stirred-tank reactor is considered as the test case.
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Title: A COMPARATIVE-STUDY OF TOOLS FOR ASSESSING THE EFFECTS OF FORCED PERIODIC OPERATION OF CATALYTIC REACTORS
Creator: Ozgulsen, F., Rigopoulos, K. R., Cinar, A.
Date: 1992
Publisher: GORDON BREACH SCI PUBL LTD
Description: Two methods for assessing the effects of forced periodic catalytic reactor operation are presented. The vibrational control method is an...
Show moreTwo methods for assessing the effects of forced periodic catalytic reactor operation are presented. The vibrational control method is an analytical technique which evaluates the effects of high frequency forcing of system parameters by the method of averaging. The second technique is a numerical tool based on a shooting algorithm. These methods are capable of handling multiple input forcing and various shapes of forcing functions. Both methods are applied to isothermal, adiabatic and nonadiabatic operation of an internal recycle reactor in which the catalytic oxidation of ethylene takes place. The basic features of both techniques are discussed and the results obtained by using these methods are compared. Effects of single and multiple input parameter forcing are investigated. Experimental verification of the theoretical results is also performed for the isothermal case.
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